Issue |
Europhys. Lett.
Volume 38, Number 5, May II 1997
|
|
---|---|---|
Page(s) | 323 - 328 | |
Section | General | |
DOI | https://doi.org/10.1209/epl/i1997-00246-4 | |
Published online | 01 September 2002 |
The relevance of Pólya's random-walk problem for the single-species reaction-diffusion system
International Centre of Theoretical Physics, Condensed Matter Section, P.O.Box 586, 34100 Trieste, Italy
Theoretische Polymerphysik - Rheinstr. 12, D-79104 Freiburg, Germany
Received:
6
September
1996
Accepted:
8
April
1997
The diffusion-limited reactions
and
in dimension
d > 2 are reconsidered
from the point of view of the random-walk
theory.
It is pointed out that Pólya's theorem on the returning probability
of a random walker to the origin, which would imply a probability
less than one
for the meeting of two typical particles, would predict
the possibility of a state in which the reaction seems to
have spontaneously ceased, in contradiction with the very well
known asymptotic
for the particles population of
these reactions.
In fact, a given condition is presented, in which
the relative particle number N(t)/N(0) decays to a
non-vanishing constant. The condition is that the
initial distribution of particles in the d-dimensional space has a
dimension γ, such that
.
PACS: 05.40.+j – Fluctuation phenomena, random processes, and Brownian motion / 82.20.Mj – Nonequilibrium kinetics
© EDP Sciences, 1997
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