Volume 68, Number 3, November 2004
|Page(s)||377 - 383|
|Section||Atomic and molecular physics|
|Published online||09 October 2004|
Low-energy positron scattering: Modelling the formation of bound states in deformed polyatomic molecules
Dipartimento di Chimica, Università di Roma “La Sapienza” and INFM Piazzale A. Moro 5, 00185 Roma, Italy
Corresponding author: firstname.lastname@example.org
Accepted: 10 September 2004
Quantum calculations are carried out to evaluate the scattering length A0 for low-energy positron collisions with gaseous acetylene molecules which are being “distorted” in their vibrational mode during the scattering. As the molecular structure undergoes increasingly larger distortions of that bending mode, the clear signature of a metastable state (change of sign for A0) appears at bending deformation of about from the linear geometry. The effects of such state on the size of the annihilation parameters of the title molecule are evaluated and the implications for larger polyatomics are discussed.
PACS: 34.85.+x – Positron scattering / 36.10.Dr – Positronium, muonium, muonic atoms and molecules / 34.50.Ez – Rotational and vibrational energy transfer
© EDP Sciences, 2004
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