Issue |
Europhys. Lett.
Volume 66, Number 6, June 2004
|
|
---|---|---|
Page(s) | 861 - 867 | |
Section | Condensed matter: electronic structure, electrical, magnetic, and optical properties | |
DOI | https://doi.org/10.1209/epl/i2004-10033-9 | |
Published online | 01 June 2004 |
Resonant photon absorption in the low-spin molecule
1
Laboratoire Louis Néel, associé à l'UJF, CNRS BP 166, 38042 Grenoble Cedex 9, France
2
Facultät für Chemie, Universitat Bielefeld - D-3300501 Bielefeld, Germany
3
Laboratoire de Photonique et de Nanostructures, CNRS - 91460 Marcoussis, France
Received:
4
February
2004
Accepted:
15
April
2004
Resonant photon absorption in the GHz range was observed via
low-temperature micro-SQUID magnetization measurements of the spin
ground state of the molecular complex
. A
simple single-molecule interpretation is proposed. The line width
essentially results from intra-molecular hyperfine interaction.
The results point out that observing Rabi oscillations in
molecular nanomagnets requires well-isolated low-spin systems and
high radiation power.
PACS: 75.45.+j – Macroscopic quantum phenomena in magnetic systems / 75.50.Xx – Molecular magnets / 75.60.Ej – Magnetization curves, hysteresis, Barkhausen and related effects
© EDP Sciences, 2004
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